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ʻO ka hoʻopili ʻana o nā hoʻonohonoho atomic, ʻoi aku ka degere o ka maʻi (DOD) o nā amorphous solids me nā waiwai, he wahi koʻikoʻi o ka hoihoi i ka ʻepekema waiwai a me nā mea condensed physics ma muli o ka paʻakikī o ka hoʻoholo ʻana i nā kūlana kūpono o nā atom i ʻekolu-dimensional. hale1,2,3,4., He mea pohihihi kahiko, 5. No keia hopena, ua haawi mai na nenee 2D i ka ike i ka mea pohihihi ma ka ae ana i na mea a pau e hoike pololei ia 6,7.ʻO ke kiʻi pololei ʻana o kahi monolayer amorphous o carbon (AMC) i ulu ʻia e ka laser deposition e hoʻonā i ka pilikia o ka hoʻonohonoho atomic, e kākoʻo ana i ka ʻike hou o nā crystallites i loko o nā paʻa aniani e pili ana i ka manaʻo o ka ʻupena8.Eia nō naʻe, ʻaʻole maopopo ka pilina kumu ma waena o ka hoʻokumu ʻana o ka unahi atomic a me nā waiwai macroscopic.Eia mākou e hōʻike maʻalahi i ka DOD a me ka conductivity i nā kiʻi ʻoniʻoni AMC ma o ka hoʻololi ʻana i ka mahana ulu.ʻO ka mea nui, ʻo ka wela o ka paepae pyrolysis ke kī nui no ka ulu ʻana i nā AMC conductive me kahi ʻano like ʻole o ka lele ʻana o ka medium order jumps (MRO), aʻo ka hoʻonui ʻana i ka mahana ma 25 ° C ke kumu e nalowale ai nā AMC i ka MRO a lilo i insulating uila, e hoʻonui ana i ke kūpaʻa o ka lau. mea i 109 manawa.Ma waho aʻe o ka nānā ʻana i nā nanocrystallites i hoʻopaʻa ʻia i loko o nā ʻenehana hoʻomau mau, ua hōʻike ʻia ka microscopy electron hoʻonā atomika i ka hele ʻana o ka MRO a me ka density nanocrystallite pili i ka mahana, ʻelua mau ʻāpana kauoha i manaʻo ʻia no ka wehewehe piha ʻana o DOD.Hoʻokumu ka helu helu helu i ka palapala conductivity ma ke ʻano he hana o kēia mau ʻāpana ʻelua, pili pono i ka microstructure i nā waiwai uila.ʻO kā mākou hana he hana koʻikoʻi i ka hoʻomaopopo ʻana i ka pilina ma waena o ke ʻano a me nā waiwai o nā mea amorphous ma kahi pae kumu a paʻa i ke ala no nā mea uila e hoʻohana ana i nā mea amorphous ʻelua.
Loaʻa nā ʻikepili kūpono a pau i hana ʻia a/a i ʻike ʻia i loko o kēia noiʻi mai nā mea kākau ma muli o ke noi kūpono.
Loaʻa ke code ma GitHub (https://github.com/vipandyc/AMC_Monte_Carlo; https://github.com/ningustc/AMCProcessing).
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Kākoʻo ʻia kēia hana e ka National Key R&D Program o Kina (2021YFA1400500, 2018YFA0305800, 2019YFA0307800, 2020YFF01014700, 2017YFA0206300), ka National Natural Science Foundation 18, 18, U3, 19 4001, 22075001, 11974024, 11874359, 92165101, 11974388, 51991344) , Beijing Natural Science Foundation (2192022, Z190011), Beijing Distinguished Young Scientist Program (BJJWZYJH01201914430039), Guangdong Provincial Key Area Research and Development Program (2019B010934001), Chinese Academy of Sciences Strategic Pilot Program, Grant No.0 X0DB Program, Grant No. ʻO ka Frontier Plan of Key ʻepekema noiʻi (QYZDB-SSW-JSC019).Mahalo nui ʻo JC i ka Beijing Natural Science Foundation o Kina (JQ22001) no kā lākou kākoʻo.Mahalo nui ʻo LW i ka Association for Promoting Youth Innovation of the Chinese Academy of Sciences (2020009) no kā lākou kākoʻo.ʻO kahi hapa o ka hana i hana ʻia i loko o ka mīkini paʻa ikaika ikaika o ka High Magnetic Field Laboratory o ka Chinese Academy of Science me ke kākoʻo o ka Anhui Province High Magnetic Field Laboratory.Hāʻawi ʻia nā kumuwaiwai e ka Peking University supercomputing platform, Shanghai supercomputing center a me Tianhe-1A supercomputer.
Эти авторы внесли равный вклад: Huifeng Tian, ​​​​Yinhang Ma, Zhenjiang Li, Mouyang Cheng, Shoucong Ning.
Huifeng Tian, ​​​​Zhenjian Li, Juijie Li, PeiChi Liao, Shulei Yu, Shizhuo Liu, Yifei Li, Xinyu Huang, Zhixin Yao, Li Lin, Xiaoxui Zhao, Ting Lei, Yanfeng Zhang, Yanlong Hou a me Lei Liu
Kula o Physics, Vacuum Physics Key Laboratory, University of Chinese Academy of Sciences, Beijing, Kina
Keʻena ʻepekema ʻenehana a me ʻenekinia, National University of Singapore, Singapore, Singapore
Beijing National Laboratory of Molecular Sciences, School of Chemistry and Molecular Engineering, Ke Kulanui o Peking, Beijing, Kina
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing, Kina